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Degradation of Azo Dye (Direct Red 89) Using H2o2/Periodate Process-Parameter Optimization and Mixture Composition Evaluation Publisher Pubmed



Riahi Zaniani A1, 2 ; Taheri E1 ; Fatehizadeh A1 ; Mohammadimoghadam F3, 4 ; Movahedian Attar H1 ; Bina B1 ; Aminabhavi TM5, 6, 7
Authors
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Authors Affiliations
  1. 1. Department of Environmental Health Engineering, School of Health, Isfahan University of Medical Sciences, Isfahan, Iran
  2. 2. Research Committee, School of Health, Isfahan University of Medical Sciences, Isfahan, Iran
  3. 3. Department of Environmental Health Engineering, School of Health, Shahrekord University of Medical Sciences, Shahrekord, Iran
  4. 4. Social Determinants of Health Research Center, Shahrekord University of Medical Sciences, Shahrekord, Iran
  5. 5. Center for Energy and Environment, School of Advanced Sciences, KLE Technological University, Hubballi, 580031, India
  6. 6. University Center for Research & Development (UCRO), Chandigarh University, Punjab, Mohali, 140 413, India
  7. 7. Korea University, Seoul, 02841, South Korea

Source: Chemosphere Published:2025


Abstract

As a fast and efficient process, a periodate (PI)-based advanced oxidation process was used to degrade direct red 89 (DR89), wherein hydrogen peroxide (H2O2) was employed to activate PI (H2O2/PI process) to investigate the effect of operating parameters and mixture composition. The PI was efficiently activated by H2O2 to degrade 67% of DR89 within 1 min. Acidic pH was more favorable to high-efficiency degradation than the basic pH; at pH 3 degradation rate was 94.31%, while it was only 20.92% at pH 11. The degradation rates were further enhanced with increasing H2O2 and PI dose up to certain optimum values, later it decreased which was dependent upon the amount of hydroxyl (●OH) and iodyl (IO3●) radicals produced. The quenching experiments suggested that IO3●, ●OH, 1O2, and O2●− are the predominant reactive species during H2O2/PI process, while O2●− radicals are the primary precursor of other reactive oxygen species. The results of this study suggested that H2O2/PI is the efficient and rapid treatment method to degrade persistent organic pollutants (POPs) from polluted wastewater sources. © 2024 Elsevier Ltd
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